Confinement-induced ultrafast conductivity in 2D perovskites resolved by correlative terahertz-NIR spectroscopy

Lion Krüger, Fabian Brütting, Michael Baumann, Moritz B. Heindl, Maximilian Spies, Anna Köhler, Alexander J. C. Kühne, and Georg Herink

Quantum wells made of quasi two-dimensional organic–inorganic hybrid perovskites (2D-PKs) offer a high degree of flexibility in tailoring optoelectronic properties through carrier confinement and functional interlayers. Compared to their 3D counterparts, 2D-PKs exhibit tunable photoluminescence, excitonic binding at room temperature, and enhanced structural stability. However, the dynamics of photoinduced charge carriers and their transport properties […]